Proposal for Observing XUV-Induced Rabi Oscillation Using Superfluorescent Emission

Jun Jie Cui, Yongjun Cheng, Xin Wang, Zheng Li, Nina Rohringer, Victor Kimberg, and Song Bin Zhang
Phys. Rev. Lett. 131, 043201 – Published 25 July 2023
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Abstract

Intense x-ray and extreme ultraviolet (XUV) light sources have been available for decades, however, due to weak nonlinear interaction in the XUV photon energy range, observation of Rabi oscillation induced by XUV pulse remains a very challenging experimental task. Here we suggest a scheme where photoionization of a He medium by an intense XUV pump pulse is followed by a strong population inversion and Rabi oscillation at the He+(1s3p) transition and is accompanied by superfluorescence (SF) of the 7.56 eV pulse at the He+(3p2s) transition. Our numerical simulations show that the Rabi oscillation at the He+(1s3p) transition induced by an XUV pulse with photon energy 48.36 eV results in significant signatures in the SF spectra, allowing us to identify and characterize the XUV induced Rabi-oscillatory regime. The proposed scheme provides a sensitive tool to monitor and control ultrafast nonlinear dynamics in atoms and molecules triggered by intense XUV.

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  • Received 28 February 2023
  • Accepted 2 June 2023

DOI:https://doi.org/10.1103/PhysRevLett.131.043201

© 2023 American Physical Society

Physics Subject Headings (PhySH)

Atomic, Molecular & Optical

Authors & Affiliations

Jun Jie Cui1, Yongjun Cheng1, Xin Wang1, Zheng Li2,3,4, Nina Rohringer5, Victor Kimberg6,*, and Song Bin Zhang1,†

  • 1School of Physics and Information Technology, Shaanxi Normal University, Xi’an 710119, China
  • 2State Key Laboratory for Mesoscopic Physics and Collaborative Innovation Center of Quantum Matter, School of Physics, Peking University, Beijing 100871, China
  • 3Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan, Shanxi 030006, China
  • 4Peking University Yangtze Delta Institute of Optoelectronics, Nantong, Jiangsu 226010, China
  • 5Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY, Notkestraße 85, 22607, Hamburg, Germany
  • 6Theoretical Chemistry and Biology, Royal Institute of Technology, Stockholm 10691, Sweden

  • *kimberg@kth.se
  • song-bin.zhang@snnu.edu.cn

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Issue

Vol. 131, Iss. 4 — 28 July 2023

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